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Molécules En Interaction Avec Des Nanoparticules Métalliques

Molécules En Interaction Avec Des Nanoparticules Métalliques

          
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About the Book

Nous avons mis en évidence le rôle de la forme et de la taille des NP ainsi que de l'épaisseur de la couche d'oxyde sur l'interaction entre NP et molécule de CO, par des expériences fondamentales capables de différentier les sites d'adsorption. Des expériences pompe-sonde nous ont permis de sonder la dynamique d'interaction des électrons excités dans les NP avec les molécules. Une analyse combinée par LEED et STM nous a permis de déterminer les meilleures conditions de croissance du film de MgO. Par la suite des NP de palladium ont été épitaxiées sur ce film. Les spectres SFG montre une forte dépendance de la fréquence de vibration avec la taille des NP et le taux de couverture en CO. Les expériences pompe sonde montrent que la particule est découplé de l´excitation électronique quand l'épaisseur de MgO dépasse 10 ML. On observe clairement un effet de taille sur l'efficacité de l'excitation électronique des NP sur les molécules de CO, qui diminue avec la taille des NP. Ceci montre que le confinement des électrons dans la particule a davantage pour effet d'augmenter la vitesse de relaxation électronique vers les phonons, que d'exciter plus efficacement les molécules adsorbées.


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Product Details
  • ISBN-13: 9783838180243
  • Publisher: Univ Europeenne
  • Binding: Paperback
  • Language: French
  • Returnable: N
  • Spine Width: 15 mm
  • Width: 152 mm
  • ISBN-10: 3838180240
  • Publisher Date: 28 Feb 2018
  • Height: 229 mm
  • No of Pages: 264
  • Series Title: Omn.Univ.Europ.
  • Weight: 394 gr


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