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Kontrollierte Eduktzufuhr in Membranreaktoren Zur Optimierung Der Ausbeute Gewunschter Produkte in Parallel- Und Folgereaktionen

Kontrollierte Eduktzufuhr in Membranreaktoren Zur Optimierung Der Ausbeute Gewunschter Produkte in Parallel- Und Folgereaktionen

          
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About the Book

In dieser Arbeit wurde die optimale Dosierung eines Eduktes entlang von Rohrreaktoren mit dem Ziel der Ausbeutemaximierung eines Zielproduktes sowohl theoretisch als auch experimentell untersucht. Ausgehend von einem isothermen und isobaren Plug-Flow-Reaktormodell zur Beschreibung einer Reihenschaltung von L Rohrreaktoren mit einer diskreten Eduktzugabe am Eintritt jeder Stufe und/oder einer verteilten Dosierung uber die Reaktorwande innerhalb der einzelnen Stufen wurden zunachst optimale Edukteinspeisungen theoretisch mit Hilfe von analytischen Losungen fur ausgewahlte Spezialfalle, mit dem Maximumprinzip sowie mit einem SQP-Algorithmus analysiert. Fur die experimentellen Untersuchungen hinsichtlich der verteilten Eduktzufuhr wurden ein einstufiger Membranreaktor zur gleichmassigen Eduktdosierung sowie eine Reihenschaltung bestehend aus 3 Membranreaktoren zur Einstellung von unterschiedlichen Dosierprofilen aufgebaut. Zur Eduktverteilung wurden in den einzelnen Membranreaktoren rohrformige asymmetrische Keramikmembranen mit einer abschliessenden gamma -Al_2O_3-Schicht eingesetzt. Als Modellreaktion wurde die oxidative Dehydrierung von Ethan zu Ethylen unter Verwendung eines VO_x/gamma -Al_2O_3-Katalysators gewahlt. Mit Hilfe der Membranreaktorkonfigurationen konnten die Auswirkungen der Sauerstoffverteilung entlang des Reaktors auf die Selektivitat des gewunschten Produktes Ethylen und auf den Umsatz des am Reaktoreintritt zugeleiteten Eduktes Ethan eindeutig demonstriert und erlautert werden.


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Product Details
  • ISBN-13: 9783832505356
  • Publisher: Logos Verlag Berlin
  • Binding: Paperback
  • Language: German
  • Returnable: N
  • Spine Width: 0 mm
  • Width: 210 mm
  • ISBN-10: 3832505350
  • Publisher Date: 19 Apr 2004
  • Height: 296 mm
  • No of Pages: 190
  • Series Title: German
  • Weight: 700 gr

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Kontrollierte Eduktzufuhr in Membranreaktoren Zur Optimierung Der Ausbeute Gewunschter Produkte in Parallel- Und Folgereaktionen
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