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Festphasensynthese Neuartiger Molekularer Transporter Und Funktioneller Peptoide

Festphasensynthese Neuartiger Molekularer Transporter Und Funktioneller Peptoide

          
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About the Book

Gezielter molekularer Transport stellt ein probates Mittel zum effizienten Einsatz bioaktiver oder pharmazeutischer Wirkstoffe dar. Die vorliegende Dissertation befasst sich mit einer Klasse peptidomimetischer Transporter, den sog. Peptoiden, welche sich von zellpenetrierenden Peptidtransportern (CPPs) ableiten lassen. In dieser Arbeit wurde ein neuer Cyclooctinlinker fur die Festphasensynthese von Peptoiden eingesetzt, welcher eine einfache und metallfreie Anbindung von Aziden und damit auch eine postsynthetische Modifikation der Transporter erlaubt. Zusatzlich wurden Peptoidtransporter mit verschiedenen, neuartigen Fluorophoren konjugiert, um deren Potential in zellbiologischen Untersuchungen zu untermauern. Zu den eingesetzten Fluorophoren zahlen, neben den bereits etablierten Cyaninen und Rhodaminen, die BOBIPY- und TADF-Farbstoffe. Daruber hinaus wurde ein wasserlosliches, fluoreszentes Single Chain Nanopartikelkonjugat auf der Basis eines Acrylsaurepolymers dargestellt, welches auf seine Eigenschaften als molekularer Transporter getestet werden soll. Des Weiteren wurden zwei Substanzbibliotheken mit je 16 literaturunbekannten Peptoiden synthetisiert. Mit Hilfe einer Bibliothek lipophiler Transporter konnen die Grenzen der Lipophilie in der Gestaltung von Peptoidtransportern sowie deren antimikrobielle Wirkungsweise getestet werden. Eine Bibliothek aus Glycopeptoiden zielt neben einer Zellgangigkeit auch auf mogliche bioaktive Wirkungsweisen. In einem letzten Teil wurde ein alternatives Transportsystem fur den Wirkstofftransport von Paclitaxel vorgestellt. Es gelang, uber zwei Syntheserouten eine orthogonal geschutzte Folsaure darzustellen, welche Teil eines oral anwendbaren Wirkstoffs sein wird.


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Product Details
  • ISBN-13: 9783832547905
  • Publisher: Logos Verlag
  • Publisher Imprint: Logos Verlag Berlin
  • Height: 210 mm
  • No of Pages: 245
  • Series Title: Beitrage Zur Organischen Synthese
  • Weight: 700 gr
  • ISBN-10: 3832547908
  • Publisher Date: 15 Nov 2018
  • Binding: Paperback
  • Language: German
  • Returnable: N
  • Spine Width: 0 mm
  • Width: 145 mm


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