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Calix[4]arènes polyphosphorylés pour la décorporation des actinides

Calix[4]arènes polyphosphorylés pour la décorporation des actinides

          
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About the Book

Le programme "Toxicologie Nucleaire et Environnementale" développé avec le CEA et le CNRS, nous avons développé de nouvelles molécules destinées à la décorporation de l'uranium en cas de contamination accidentelle, ces ligands devant être compatibles avec les milieux biologiques et non-toxiques. Nous avons utilisé les propriétés chélatantes des groupements bisphosphonates et la capacité de préorganisation des calix[4]arènes. Nous avons fait varier le bras espaceur entre le support topologique et la fonction complexante sur la partie "upper rim" du calixarène et avons synthétisé le premier calix[4]arène greffé par un bisphosphonate sur la fonction phénol de la partie "lower rim". L'introduction du groupe hydroxyméthylène bisphosphonate a été possible en utilisant le tris(triméthylsilyl)phosphite suivi d'une hydrolyse. Nous avons ensuite déterminé leurs constantes d'affinité vis à vis du cation uranyle. Nous avons montré que les calix[4]arènes substitués sur le "upper rim" sont de bons ligands pour l'uranium. Des études préliminaires de toxicité cellulaire sur des cellules hépatiques ont été réalisées, ces ligands ne sont pas toxiques à 1 mM.


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Product Details
  • ISBN-13: 9786131545221
  • Publisher: Omniscriptum
  • Publisher Imprint: Omniscriptum
  • Height: 229 mm
  • No of Pages: 168
  • Series Title: Omn.Univ.Europ.
  • Weight: 258 gr
  • ISBN-10: 6131545227
  • Publisher Date: 28 Feb 2018
  • Binding: Paperback
  • Language: French
  • Returnable: N
  • Spine Width: 10 mm
  • Width: 152 mm


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